Abstract:East Asian region is one of the largest monsoon regions in the world,and East Asian winter monsoon(EAWM) plays an important role in the regional climate.Anthropogenic sulfate and black carbon(BC) are most important radiation active aerosols in East Asia.The interaction between aerosols and East Asian monsoon climate has received more and more attention in recent years.In this study,the impact of increase in anthropogenic aerosols on EAWM over eastern China are investigated using the NCAR Community Atmospheric Model version 5.1(CAM5.1),a state-of-the-art climate model considering aerosol direct,semi-direct and indirect effects.The effects of increase in anthropogenic sulfate,BC and both of them on EAWM are decomposed from different sensitivity simulations by changing anthropogenic aerosol emission sources in eastern China,and the experiments differed only in the aerosol and precursor gas emissions.CAM5.1 can generally capture the main features of winter atmospheric circulation in East Asia.
In winter,the direct and 1st indirect effects of sulfate reduce the solar flux reaching the surface,leading to a reduction of air temperature of surface and low troposphere and an increase of sea level pressure over land.Adjustments in surface temperature and pressure fields result in a weakened wind field above 925 hPa.The gradient of pressure between land and sea is increased,which enhances EAWM.The large-scale precipitation in southern China is reduced by the 2nd indirect effects of sulfate,and the convective precipitation is reduced in northern China,which is caused by the changed circulation.In winter,the effects of BC reduce the solar flux reaching the surface,and increase the solar flux in the atmosphere by absorbing.The surface air temperature has an insignificant reduction because the semi-direct effects of BC partly offset the direct.The heating of the low troposphere leads to the enhanced convection and the increased convective precipitation in southern China.The changed circulation results in temperature increase in troposphere over China.Adjustments in surface temperature and pressure fields result in an enhanced north wind in northern China and a weakened wind field in southern China above 925 hPa.The effects of BC result to an enhanced(a weakened) EAWM in northern(southern) China.The effects of BC on cloud are different from sulfate,which come from the feedback of semi-direct effect and the changed circulation.The effects of total anthropogenic aerosols(both sulfate and BC aerosols) result in a weaker reduction of air temperature in winter,which are the common result of two kinds of aerosols.The convective and large-scale precipitations are both reduced in northern China,and the convective precipitation is increased in southern China.The changes in surface temperature and pressure fields also result in an enhanced wind field in northern China and a weakened wind field in southern China above 925 hPa.The effects of total anthropogenic aerosols also result in an enhanced(a weakened) EAWM in northern(southern) China.The effects of total anthropogenic aerosols on monsoon are not simply a linear summation between the two types of aerosols.